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Grateful Dead - Dark Star (Live at the Fillmore West San Francisco, 1969) (2001 Remaster)
As for 60s American psych (which will never be as psych as Hawkwind and Gong, given the omnipresent influence of the blues), Dark Star and In a Gadda da Vida are my favorite jams that best encapsulate the genre.
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Grateful DeadLive/Dead
Live - 10 november 1969

Each song lets the artists go into improvisations, but simultaneously they remain united as if they were an aerobatic squadron painting the sky with their smoke trails. EatherSun